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Low temperature conversion of toluene to methane using dielectric barrier discharge reactor

Lookup NU author(s): Faisal Saleem, Professor Adam Harvey, Dr Kui Zhang

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This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License (CC BY-NC-ND).


Abstract

© 2019 Elsevier Ltd A dielectric barrier discharge reactor was used to convert toluene (tar analogue) into methane (>90%). This study showed that wall temperature and plasma power played key roles on the product distribution. At ambient conditions, solid formation was observed inside the reactor at all tested powers (50–85 W). The maximum selectivity to lower hydrocarbon (C 1 -C 6 ) was 63% at 85 W. However, complete conversion of the toluene to lower hydrocarbons was seen at power (75 W), when the surrounding temperature raised to 200 °C. Significant increase in selectivity also observed at 50 W, where selectivity increased from 35% to 84%, at 200 °C. The selectivity to various lower hydrocarbons was strongly dependent upon power. Methane showed maximum selectivity >90% at 85 W and 200 °C, whereas at 50 W the other hydrocarbons >C 1 were >40% along with methane. The selectivity of C 2 -C 6 started to decrease when increasing power due to increased cracking into methane.


Publication metadata

Author(s): Saleem F, Harvey A, Zhang K

Publication type: Article

Publication status: Published

Journal: Fuel

Year: 2019

Volume: 248

Pages: 258-261

Print publication date: 15/07/2019

Online publication date: 01/04/2019

Acceptance date: 28/02/2019

Date deposited: 13/05/2019

ISSN (print): 0016-2361

ISSN (electronic): 1873-7153

Publisher: Elsevier Ltd

URL: https://doi.org/10.1016/j.fuel.2019.02.137

DOI: 10.1016/j.fuel.2019.02.137


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Funding

Funder referenceFunder name
EP/J017302/1EPSRC
University of Engineering and Technology Lahore, Pakistan

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