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Prediction of sorption enhanced steam methane reforming products from machine learning based soft-sensor models

Lookup NU author(s): Dr Yongliang YanORCiD

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This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License (CC BY-NC-ND).


Abstract

Carbon dioxide-abated hydrogen can be synthesised via various processes, one of which is sorption enhanced steam methane reforming (SE-SMR), which produces separated streams of high purity H2 and CO2. Properties of hydrogen and the sorbent material hinder the ability to rapidly upscale SE-SMR, therefore the use of artificial intelligence models is useful in order to assist scale up. Advantages of a data driven soft-sensor model over thermodynamic simulations, is the ability to obtain real time information dependent on actual process conditions. In this study, two soft sensor models have been developed and used to predict and estimate variables that would otherwise be difficult direct measured. Both artificial neural networks and the random forest models were developed as soft sensor prediction models. They were shown to provide good predictions for gas concentrations in the reformer and regenerator reactors of the SE-SMR process using temperature, pressure, steam to carbon ratio and sorbent to carbon ratio as input process features. Both models were very accurate with high R2 values, all above 98%. However, the random forest model was more precise in the predictions, with consistently higher R2 values and lower mean absolute error (0.002-0.014) compared to the neural network model (0.005-0.024).


Publication metadata

Author(s): Nkulikiyinka P, Yan Y, Güleç F, Manovic V, Clough P

Publication type: Article

Publication status: Published

Journal: Energy and AI

Year: 2020

Volume: 2

Print publication date: 04/11/2020

Online publication date: 11/11/2020

Acceptance date: 06/11/2020

Date deposited: 24/02/2021

ISSN (electronic): 2666-5468

Publisher: Elsevier BV

URL: https://doi.org/10.1016/j.egyai.2020.100037

DOI: 10.1016/j.egyai.2020.100037


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Funding

Funder referenceFunder name
UK Engineering and Physical Sciences Research Council Doctoral Training Partnership (EPSRC DTP) grant No. EP/R513027/1.

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