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Thermodiffusively-unstable lean premixed hydrogen-methane blends: Phenomenology and empirical modelling

Lookup NU author(s): Dr Edward HuntORCiD, Dr Arnab Moitro, Dr Andrew AspdenORCiD

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This work is licensed under a Creative Commons Attribution 4.0 International License (CC BY 4.0).


Abstract

This paper considers direct numerical simulation of hydrogen–methane blends in three-dimensional freely-propagating and turbulent flames using the canonical flame-in-a-box configuration. Previous work has developed empirical models for mean local flame speed and thickness in two- and three-dimensional freely-propagating flames, as well as a Karlovitz-dependent modification to capture the exaggeration of thermodiffusive response by turbulence; more recently, a modification to the instability parameter was demonstrated for hydrogen–methane blends two-dimensional freely-propagating flames. The present paper first considers phenomenology of premixed flames of fuel blends where one component is thermodiffusively unstable, and shows that there are effectively two flames, correlated with local curvature. In regions of positive curvature (centre of curvature in the products), the usual thermodiffusive response is observed; diffusive focussing of hydrogen results in flames locally thinner and faster. For the fuel blend, the other component (in this case methane) is left behind, and burns more slowly in the negatively-curved regions (where extinction channels would be found in unblended hydrogen flames). The dual-flame nature of the burning means that the choice of progress variable becomes more important; the selected isosurfaces based on hydrogen and temperature did not correlate well with the negatively-curved heat release associated with methane consumption, and so a blend-based progress variable was required. Consequently, the blend-based flame surface area was up to 50% higher than the other surfaces, resulting in lower mean local flame speeds. Joint probability density functions of local flame speed and curvature highlight the dual-flame nature, with high flame speeds correlating positively with curvature and a second region of low level burning at negative curvatures. The empirical models are shown to work well in three dimensions; the modification to the instability parameter for blends is independent of dimension. An additional factor was required in the turbulent flame speed model to reduce the turbulent contribution to local flame speed as the hydrogen content goes to zero. The resulting empirical model is shown to work remarkably well, and provides a prediction of mean local flame speed for turbulent thermodiffusively-unstable lean premixed hydrogen–methane blends, which can be evaluated simply from one-dimensional flame simulations alone.


Publication metadata

Author(s): Hunt EF, Moitro A, Aspden AJ

Publication type: Article

Publication status: Published

Journal: Combustion and Flame

Year: 2026

Volume: 286

Print publication date: 01/04/2026

Online publication date: 05/02/2026

Acceptance date: 27/01/2026

Date deposited: 26/01/2026

ISSN (print): 0010-2180

ISSN (electronic): 1556-2921

Publisher: Elsevier Inc.

URL: https://doi.org/10.1016/j.combustflame.2026.114845

DOI: 10.1016/j.combustflame.2026.114845

ePrints DOI: 10.57711/sf8n-q232


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Funding

Funder referenceFunder name
EPSRC
EP/W034506/1

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